Article: Thermodynamic characterization of interpenetrating polymer networks.

INTRODUCTION

Originally, interpenetrating polymer networks (IPN) were conceived as chemically homogeneous (on a sufficiently large structural scale), binary systems that could be conveniently prepared by swelling the first loosely crosslinked component in a suitably chosen monomer and subsequent crosslinking of the latter (1, 2). Conceptually, this procedure of "chemical" blending might avoid the eventual phase separation that is typical of "physical" blending of linear polymers (3, 4), a result of topological constraints (permanently entangled, chemically different macrocycles) on IPN unmixing (5, 6). However, it was realized fairly soon that the overwhelming ...

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